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RAS Chemistry & Material ScienceЖурнал прикладной химии Russian Journal of Applied Chemistry

  • ISSN (Print) 0044-4618
  • ISSN (Online) 3034-5545

ELECTROCHEMICAL REDUCTION OF GASES USING GAS DIFFUSION ELECTRODES: A REVIEW OF RECENT ADVANCES

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PII
S30345545S0044461825070063-1
DOI
10.7868/S3034554525070063
Publication type
Review
Status
Published
Authors
N. V. Maltseva
  • Affiliation:
    Novosibirsk State University
    G. K. Boreskov Institute of Catalysis SB RAS
P. A. Nikolaichuk
  • Occupation: Cand. Sci. (Chem.)
  • Affiliation: Novosibirsk State University
M. V. Lebedeva
  • Occupation: Cand. Sci. (Chem.)
  • Affiliation:
    Novosibirsk State University
    G. K. Boreskov Institute of Catalysis SB RAS
D. V. Kozlov
  • Occupation: Dr. Sci. (Chem.)
  • Affiliation:
    Novosibirsk State University
    G. K. Boreskov Institute of Catalysis SB RAS
Volume/ Edition
Volume 98 / Issue number 7-8
Pages
459-472
Abstract
Practical application of electrochemical gas reduction to obtain valuable products is hampered by slow mass transfer and low solubility of gases in most electrolytes. When using gas diffusion electrodes, mass transfer of gas to the electrode surface is improved, which helps maintain a high concentration of the reagent near the catalyst layer and allows increasing the product yield by tens of times. The article presents a review of works devoted to the electrochemical reduction of O, CO, CO, N, NO using cells with a gas diffusion electrode. Information on electrode materials and process characteristics is provided. In the CO reduction reaction on electrode materials based on Au, Ag, Zn, Co, Fe, Ni, the main product is CO; when using materials based on Bi, Pb, Sb, In, Sn, HCOOH is formed with high selectivity. Lower hydrocarbons, alcohols and carboxylic acids can be obtained using electrode materials based on Cu. Reduction of O with the formation of HO occurs when using electrode materials based on C, Fe, Ti, Ag. Formation of NH during reduction of N or NO occurs when using materials based on C, Ca, Cu. Electrochemical cells with gas diffusion electrodes can be used as elements of complex systems for CO capture and processing and continuous reactors. Developments are underway on designs of electrochemical cells with two gas diffusion electrodes and electrodes with a surface area of more than 1 m. The features of gas diffusion electrode assembly, problems and ways of technology development are described. A comparison of gas electroreduction processes in systems with submerged and gas diffusion electrodes is provided.
Keywords
электровосстановление газов газодиффузионный электрод диоксид углерода моноксид углерода кислород азот моноксид азота пероксид водорода электродные материалы
Date of publication
01.01.2026
Year of publication
2026
Number of purchasers
0
Views
40

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Higher Attestation Commission

At the Ministry of Education and Science of the Russian Federation

Scopus

Scientific Electronic Library